The urgency the address high CO2 concentrations in the Earth’s atmosphere increases each day prompting collaborative efforts between industry and the science community to develop various solutions. Among these, carbon capture utilization and storage (CCUS) technologies are proven to be integral. Rooted in CO2 adsorption, carbon capture forms the cornerstone of CCUS technologies. Consequently, developing effective CO2 capture materials and designing systems capable of integrating these materials into real-world practical applications play a crucial role. In this study, one of the most promising materials for future CO2 capture technologies, Ni-MOF-74, is synthesized, characterized, and tested for CO2 adsorption capacity. Following the synthesis process Ni-MOF-74 is immobilized on acrylonitrile fabric in order to achieve a flexible and versatile structure with high CO2 capacity that can be integrated in various applications. The highest surface area and CO2 adsorption capacity achieved by the synthesized NiMOF-74 powder are 180 m2 /g and 1.98 mmol/g, respectively. Synthesized Ni-MOF-74 powder was successfully immobilized on an acrylic fabric substrate through the drip casting method. The resulting composite showed a decrease in CO2 adsorption capacity only by 8% which is promising for practical applications and a fair compromise considering that the flexible structure offers an opportunity to be utilized in a wide range of scenarios.